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It has been known for a long time that the shape of ice crystals depends on both the air temperature and the relative humidity of the environment. The relationships among these factors have been summarized in classification diagrams and are intensively referred to in the cloud physics literature. To put in perspective the atmospheric conditions in which the different ice crystal habits grow with respect to the level of saturation in the atmosphere, the vapor density excess and supersaturation with respect to ice at liquid water saturation have been included on those diagrams as a function of air temperature. Over the years, the definition of the water saturation included in those types of diagrams has been misdefined. The goal of this study is to show that an error has been introduced in the definition of the excess of water vapor with respect to ice.

Abstract The accurate measurement of snowfall is important in various fields of study such as climate variability, transportation, and water resources. A major concern is that snowfall measurements are difficult and can result in significant errors. For example, collection efficiency of most gauge–shield configurations generally decreases with increasing wind speed. In addition, much scatter is observed for a given wind speed, which is thought to be caused by the type of snowflake. Furthermore, the collection efficiency depends strongly on the reference used to correct the data, which is often the Double Fence Intercomparison Reference (DFIR) recommended by the World Meteorological Organization. The goal of this study is to assess the impact of weather conditions on the collection efficiency of the DFIR. Note that the DFIR is defined as a manual gauge placed in a double fence. In this study, however, only the double fence is being investigated while still being called DFIR. To address this issue, a detailed analysis of the flow field in the vicinity of the DFIR is conducted using computational fluid dynamics. Particle trajectories are obtained to compute the collection efficiency associated with different precipitation types for varying wind speed. The results show that the precipitation reaching the center of the DFIR can exceed 100% of the actual precipitation, and it depends on the snowflake type, wind speed, and direction. Overall, this study contributes to a better understanding of the sources of uncertainty associated with the use of the DFIR as a reference gauge to measure snowfall.

Abstract Understanding the responses of lake systems to past climate change and human activity is critical for assessing and predicting the fate of lake carbon (C) in the future. In this study, we synthesized records of the sediment accumulation from 82 lakes and of C sequestration from 58 lakes with direct organic C measurements throughout China. We also identified the controlling factors of the long‐term sediment and C accumulation dynamics in these lakes during the past 12 ka (1 ka = 1000 cal yr BP ). Our results indicated an overall increasing trend of sediment and C accumulation since 12 ka, with an accumulation peak in the last couple of millennia for lakes in China, corresponding to terrestrial organic matter input due to land‐use change. The Holocene lake sediment accumulation rate ( SAR ) and C accumulation rate ( CAR ) averaged (mean ± SE ) 0.47 ± 0.05 mm yr −1 and 7.7 ± 1.4 g C m −2  yr −1 in China, respectively, comparable to the previous estimates for boreal and temperate regions. The SAR for lakes in the East Plain of subtropical China (1.05 ± 0.28 mm yr −1 ) was higher than those in other regions ( P  <   0.05). However, CAR did not vary significantly among regions. Overall, the variability and history of climate and anthropogenic interference regulated the temporal and spatial dynamics of sediment and C sequestration for lakes in China. We estimated the total amount of C burial in lakes of China as 8.0 ± 1.0 Pg C. This first estimation of total C storage and dynamics in lakes of China confirms the importance of lakes in land C budget in monsoon‐influenced regions.

Dynamic global vegetation models (DGVMs) typically track the material and energy cycles in ecosystems with finite plant functional types (PFTs). Increasingly, the community ecology and modelling studies recognize that current PFT scheme is not sufficient for simulating ecological processes. Recent advances in the study of plant functional traits (FTs) in community ecology provide a novel and feasible approach for the improvement of PFT-based DGVMs. This paper reviews the development of current DGVMs over recent decades. After characterizing the advantages and disadvantages of the PFT-based scheme, it summarizes trait-based theories and discusses the possibility of incorporating FTs into DGVMs. More importantly, this paper summarizes three strategies for constructing next-generation DGVMs with FTs. Finally, the method’s limitations, current challenges and future research directions for FT theory are discussed for FT theory. We strongly recommend the inclusion of several FTs, namely specific leaf area (SLA), leaf nitrogen content (LNC), carbon isotope composition of leaves (Leaf δ 13 C), the ratio between leaf-internal and ambient mole fractions of CO 2 (Leaf C i /C a ), seed mass and plant height. These are identified as the most important in constructing DGVMs based on FTs, which are also recognized as important ecological strategies for plants. The integration of FTs into dynamic vegetation models is a critical step towards improving the results of DGVM simulations; communication and cooperation among ecologists and modellers is equally important for the development of the next generation of DGVMs.

Abstract Aim The fluctuations of atmospheric methane ( CH 4 ) that have occurred in recent decades are not fully understood, particularly with regard to the contribution from wetlands. The application of spatially explicit parameters has been suggested as an effective method for reducing uncertainties in bottom‐up approaches to wetland CH 4 emissions, but has not been included in recent studies. Our goal was to estimate spatio‐temporal patterns of global wetland CH 4 emissions using a process model and then to identify the contribution of wetland emissions to atmospheric CH 4 fluctuations. Location Global. Methods A process‐based model integrated with full descriptions of methanogenesis ( TRIPLEX‐GHG ) was used to simulate global wetland CH 4 emissions. Results Global annual wetland CH 4 emissions ranged from 209 to 245  T g CH 4 year −1 between 1901 and 2012, with peaks occurring in 1991 and 2012. There is a decreasing trend between 1990 and 2010 with a rate of approximately 0.48  T g CH 4 year −1 , which was largely caused by emissions from tropical wetlands showing a decreasing trend of 0.44  T g CH 4 year −1 since the 1970s. Emissions from tropical, temperate and high‐latitude wetlands comprised 59, 26 and 15% of global emissions, respectively. Main conclusion Global wetland CH 4 emissions, the interannual variability of which was primary controlled by tropical wetlands, partially drive the atmospheric CH 4 burden. The stable to decreasing trend in wetland CH 4 emissions, a result of a balance of emissions from tropical and extratropical wetlands, was a particular factor in slowing the atmospheric CH 4 growth rate during the 1990s. The rapid decrease in tropical wetland CH 4 emissions that began in 2000 was supposed to offset the increase in anthropogenic emissions and resulted in a relatively stable level of atmospheric CH 4 from 2000 to 2006. Increasing wetland CH 4 emissions, particularly after 2010, should be an important contributor to the growth in atmospheric CH 4 seen since 2007.

Abstract The effect of large-scale irrigation in India on the moisture budget of the atmosphere was investigated using three regional climate models and one global climate model, all of which performed an irrigated run and a natural run without irrigation. Using a common irrigation map, year-round irrigation was represented by adding water to the soil moisture to keep it at 90% of the maximum soil moisture storage capacity, regardless of water availability. For two focus regions, the seasonal cycle of irrigation matched that of the reference dataset, but irrigation application varied between the models by up to 0.8 mm day−1. Because of the irrigation, evaporation increased in all models, but precipitation decreased because of a strong decrease in atmospheric moisture convergence. A moisture tracking scheme was used to track individual evaporated moisture parcels through the atmosphere to determine where these lead to precipitation. Up to 35% of the evaporation moisture from the Ganges basin is recycling within the river basin. However, because of a decreased moisture convergence into the river basin, the total amount of precipitation in the Ganges basin decreases. Although a significant fraction of the evaporation moisture recycles within the river basin, the changes in large-scale wind patterns due to irrigation shift the precipitation from the eastern parts of India and Nepal to the northern and western parts of India and Pakistan. In these areas where precipitation increases, the relative precipitation increase is larger than the relative decrease in the areas where precipitation decreases. It is concluded 1) that the direct effects of irrigation on precipitation are small and are not uniform across the models; 2) that a fraction of up to 35% of any marginal evaporation increase (for example, due to irrigation) will recycle within the river basin; and 3) that when irrigation is applied on a large scale, the dominant effect will be a change in large-scale atmospheric flow that decreases precipitation in eastern India and increases it in western and northern India.

Abstract. A new process-based model TRIPLEX-GHG was developed based on the Integrated Biosphere Simulator (IBIS), coupled with a new methane (CH4) biogeochemistry module (incorporating CH4 production, oxidation, and transportation processes) and a water table module to investigate CH4 emission processes and dynamics that occur in natural wetlands. Sensitivity analysis indicates that the most sensitive parameters to evaluate CH4 emission processes from wetlands are r (defined as the CH4 to CO2 release ratio) and Q10 in the CH4 production process. These two parameters were subsequently calibrated to data obtained from 19 sites collected from approximately 35 studies across different wetlands globally. Being heterogeneously spatially distributed, r ranged from 0.1 to 0.7 with a mean value of 0.23, and the Q10 for CH4 production ranged from 1.6 to 4.5 with a mean value of 2.48. The model performed well when simulating magnitude and capturing temporal patterns in CH4 emissions from natural wetlands. Results suggest that the model is able to be applied to different wetlands under varying conditions and is also applicable for global-scale simulations.

Abstract. Even though dissolved organic carbon (DOC) is the most active carbon (C) cycling in soil organic carbon (SOC) pools, it receives little attention from the global C budget. DOC fluxes are critical to aquatic ecosystem inputs and contribute to the C balance of terrestrial ecosystems, but few ecosystem models have attempted to integrate DOC dynamics into terrestrial C cycling. This study introduces a new process-based model, TRIPLEX-DOC, that is capable of estimating DOC dynamics in forest soils by incorporating both ecological drivers and biogeochemical processes. TRIPLEX-DOC was developed from Forest-DNDC, a biogeochemical model simulating C and nitrogen (N) dynamics, coupled with a new DOC process module that predicts metabolic transformations, sorption/desorption, and DOC leaching in forest soils. The model was validated against field observations of DOC concentrations and fluxes at white pine forest stands located in southern Ontario, Canada. The model was able to simulate seasonal dynamics of DOC concentrations and the magnitudes observed within different soil layers, as well as DOC leaching in the age sequence of these forests. Additionally, TRIPLEX-DOC estimated the effect of forest harvesting on DOC leaching, with a significant increase following harvesting, illustrating that land use change is of critical importance in regulating DOC leaching in temperate forests as an important source of C input to aquatic ecosystems.

Abstract. Recently, two types of ice clouds (TICs) properties have been characterized using the Indirect and Semi-Direct Aerosol Campaign (ISDAC) airborne measurements (Alaska, April 2008). TIC-2B were characterized by fewer (< 10 L−1) and larger (> 110 μm) ice crystals, and a larger ice supersaturation (> 15%) compared to TIC-1/2A. It has been hypothesized that emissions of SO2 may reduce the ice nucleating properties of ice nuclei (IN) through acidification, resulting in a smaller concentration of larger ice crystals and leading to precipitation (e.g., cloud regime TIC-2B). Here, the origin of air masses forming the ISDAC TIC-1/2A (1 April 2008) and TIC-2B (15 April 2008) is investigated using trajectory tools and satellite data. Results show that the synoptic conditions favor air masses transport from three potential SO2 emission sources into Alaska: eastern China and Siberia where anthropogenic and biomass burning emissions, respectively, are produced, and the volcanic region of the Kamchatka/Aleutians. Weather conditions allow the accumulation of pollutants from eastern China and Siberia over Alaska, most probably with the contribution of acidic volcanic aerosol during the TIC-2B period. Observation Monitoring Instrument (OMI) satellite observations reveal that SO2 concentrations in air masses forming the TIC-2B were larger than in air masses forming the TIC-1/2A. Airborne measurements show high acidity near the TIC-2B flight where humidity was low. These results support the hypothesis that acidic coating on IN could be at the origin of the formation of TIC-2B.

Abstract Model simulations of the Greenland ice sheet contribution to 21st-century sea-level rise are performed with a state-of-the-art ice-sheet model (Parallel Ice Sheet Model (PISM)). The climate-forcing fields are obtained from the European Union’s Seventh Framework Programme project ice2sea, in which three regional climate models are used to dynamically downscale two scenarios (A1B and E1) from two general circulation models (ECHAM5 and HadCM3). To assess the sensitivity of the projections to the model initial state, four initialization methods are applied. In these experiments, the simulated contribution to sea-level rise by 2100 ranges from an equivalent of 0.2 to 6.8 cm. The largest uncertainties arise from different formulations of the regional climate models (0.8–3.9 cm) and applied scenarios (0.65–1.9 cm), but an important source of uncertainty is the initialization method (0.1–0.8 cm). These model simulations do not account for the recently observed acceleration of ice streams and consequent thinning rates, the changing ice discharge that may result from the spatial and temporal variability of ocean forcing, or the feedback occurring between ice-sheet elevation changes and climate forcing. Thus the results should be considered the lower limit of Greenland ice sheet contributions to sea-level rise, until such processes have been integrated into large-scale ice-sheet models.