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RÉSUMÉ: La modélisation hydrodynamique est un élément fondamental du génie hydraulique. Elle permet de créer des modèles de bassins versants et de rivières pour la prédiction des inondations. La simulation des phénomènes d'inondation est un sujet de plus en plus important dans le domaine de la recherche en hydraulique. Compte tenu des exigences d'évaluation spécifiques dans les plans d'ingénierie des risques d'inondation, la modélisation des inondations devient très importante dans le génie hydraulique. La délimitation probabiliste des zones inondables joue un rôle déterminant dans les plans d'ingénierie des risques. Cette tâche importante est réalisable à l'aide de la simulation post-inondation et de la détermination des limites de l'étendue des inondations avec leurs probabilités d'occurrence correspondantes dans les zones étudiées. ABSTRACT: Hydrodynamic modeling including watershed, river and flood modeling is a fundamental part of hydraulic engineering. In this regard, simulation of flood phenomena is an increasingly important subject in hydraulic research domain. Considering specific evaluation requirements in flood risk engineering plans, flood modeling is becoming highly important based on hydrological method (rainfall-runoff) or hydraulic parameters in Hydraulic engineering.

RÉSUMÉ: La modélisation hydrodynamique est un élément fondamental du génie hydraulique. Elle permet de créer des modèles de bassins versants et de rivières pour la prédiction des inondations. La simulation des phénomènes d'inondation est un sujet de plus en plus important dans le domaine de la recherche en hydraulique. Compte tenu des exigences d'évaluation spécifiques dans les plans d'ingénierie des risques d'inondation, la modélisation des inondations devient très importante dans le génie hydraulique. La délimitation probabiliste des zones inondables joue un rôle déterminant dans les plans d'ingénierie des risques. Cette tâche importante est réalisable à l'aide de la simulation post-inondation et de la détermination des limites de l'étendue des inondations avec leurs probabilités d'occurrence correspondantes dans les zones étudiées. ABSTRACT: Hydrodynamic modeling including watershed, river and flood modeling is a fundamental part of hydraulic engineering. In this regard, simulation of flood phenomena is an increasingly important subject in hydraulic research domain. Considering specific evaluation requirements in flood risk engineering plans, flood modeling is becoming highly important based on hydrological method (rainfall-runoff) or hydraulic parameters in Hydraulic engineering.

L'évaluation de l'impact hydrologique du changement climatique présente une importance particulière pour les bassins de la Méditerranée, qui sont très sensibles aux événements hydrologiques extrêmes. La modélisation des systèmes aussi complexes pour la gestion des ressources hydriques est un défi difficile. L'objectif global de ce travail est de contribuer au développement d'une approche de modélisation qui permette l'évaluation de l'impact hydrologique du changement climatique sur deux bassins de la Méditerranée, localisés en Sardaigne. Cette contribution se concentre sur deux sujets principaux: comprendre comment la représentation physique des modèles hydrologiques grave sur l'évaluation de l'impact hydrologique dû au changement climatique sur un bassin avec un climat semi-aride, le Rio Mannu di San Sperate, et montrer comme le modélisation avancé puisse aider à définir de mesures de modération et adaptation dans un système complexe enclin aux événements hydrique extrêmes, le Flumendosa, en conditions de changement climatique. Pour atteindre cet objectif le travail s'articule en trois phases. Les effets du changement climatique sur le bassin du Rio Mannu sont évalués à travers la comparaison des résultats de cinq modèles hydrologiques, CATchment HYdrology (CATHY), Soil and Water Assessment Tool (SWAT), TIN-based Real time Integrated Basin Simulator (tRIBS), TOPographic Kinematic APproximation and Integration-eXtended (TOPKAPI-X), and Water flow and balance Simulation Model (WASIM), en utilisant comme forçage atmosphérique les données de quatre combinaisons de modèles climatiques globaux (GCM) et régionaux (RCM). Pour évaluer les incertitudes une métrique récemment proposée est utilisée: les résultats des modèles sont comparés pendant une période de référence et future, en utilisant l'index de corrélation de Pearson et le bias de Duveiller. Même si certaines différences existent, en tout les modèles hydrologiques montrent une bonne concordance, et ils répondent de manière semblable à la réduction de la précipitation et à l'accroissement de la température prévu par les modèles climatiques. Il s'attend donc que le bassin dans l'avenir sera sujet à une réduction de la disponibilité de ressource hydrique, avec des conséquences négatives en particulier pour le secteur agricole. Une comparaison détaillée des réponses obtenue sur le même bassin avec trois modèles hydrologique à base physique avec différent degré pour ce qui concerne la représentation des procès physiques et des caractéristiques du terrain, CATHY, TOPKAPI-X, tRIBS, est effectué dans le but de tester la transférabilité des paramètres entre les trois modèles hydrologiques, avec une attention particulière sur les difficultés relevées dans les périodes de calibrage et validation. Tandis que les trois modèles ont répondu de manière semblable pendant la période de calibrage, significatives différences ont été relevées pendant la période de validation, caractérisé par un climat très sec, avec le modèle CATHY, qu'il a produit un très bas décharge. En conséquence, pour obtenir résultats satisfaisants avec le modèle CATHY, l’hypothèse de croûtage de sol a été assumée, sur la base dont la couche premier de sol a été modelée avec une conductibilité hydraulique saturée réduite. Finalement le modèle TOPKAPI-X est implémenté sur un des principaux bassins de la Sardaigne, d'importance stratégique pour le système hydrique de la région, le Flumendosa, afin d’évaluer les effets du changement climatique à plus grande échelle. Le modèle répond avec une diminution des valeurs de décharge, contenu hydrique et évapotranspiration réelle à la réduction de la précipitation et accroissement des températures prévus par les modèles climatiques en donnant aussi support à une scène future de carence de la ressource hydrique dans ce bassin de la zone Méditerranéenne.<br /><br />Assessing the hydrologic impacts of climate change is of great importance in the Mediterranean basins, which are heavily sensitive to climate variability, with significant impacts on water resources and hydrologic extremes. Modeling such complex systems to manage water resources and predict hydrologic extremes is a difficult task. The overall aim of the work described in this thesis is to bring a contribution in developing a modeling approach that allows evaluation of local hydrologic impacts of climate changes in two Mediterranean catchments located in Sardinia. This contribution revolves around two main themes: understanding how physical representation of hydrologic models can affect hydrologic impact assessment under climate change on a semi-arid basin of the Mediterranean region, the Rio Mannu catchment, and demonstrating how advanced hydrologic modeling can help in defining adaptation measures in a complex water system, the Flumendosa basin, under climate change. The work to achieve the general objective is elaborated into three stages. The effects of climate change are evaluated on the Rio Mannu catchment through comparison of the results from five hydrologic models, CATchment HYdrology (CATHY), Soil and Water Assessment Tool (SWAT), TIN-based Real time Integrated Basin Simulator (tRIBS), TOPographic Kinematic APproximation and Integration-eXtended (TOPKAPI-X), and Water flow and balance Simulation Model (WASIM), and using as atmospheric input outputs of four climate global (GCM) and regional (RCM) model combinations. In order to evaluate uncertainties, a recently proposed metric is used: climate and hydrologic models results are compared in terms of agreement with each other in reference and future periods using Pearson correlation values and Duveiller bias. Notwithstanding some differences, overall the five hydrologic models show good agreement, and they respond similarly to the reduced precipitation and increased temperatures predicted by the climate models, lending strong support to a future scenario of increased water shortages for this region of the Mediterranean, with negative consequences especially for the agricultural sector. Detailed comparison of the responses obtained with three physically based hydrologic models, but to varying degrees as regards physical processes and terrain features representation – CATHY, tRIBS, and TOPKAPI-X – on the same catchment is carried out, with the aim to test the transferability of parameters between the three hydrologic models, focusing in particular on the calibration and validation difficulties. While the three hydrologic models responded similarly during the calibration year, significant differences were found for the drier validation period for the CATHY model, which produced very low streamflow. To obtain satisfactory results for the CATHY model, an hypothesis of soil crusting was assumed and the first soil layer was modeled with a lower saturated hydraulic conductivity. Finally, the TOPKAPI-X model is applied on a large Sardinian basin prone to extreme flood events, the Flumendosa basin, to assess the hydrologic impact of climate change at much larger scale. The model responds with decreasing value of discharge, soil water content, and actual evapotranspiration to the reduced precipitation and increased temperature predicted by the climate models, lending strong support to a future scenario of increased water shortages also in this basin of the Mediterranean region.<br /><br />La valutazione dell’impatto idrologico del cambiamento climatico riveste particolare importanza per i bacini del Mediterraneo, sensibili ad eventi idrologici estremi. Modellizzare dei sistemi così complessi per la gestione della risorse idriche è una sfida difficile. L’obiettivo globale di questo lavoro è contribuire allo sviluppo di un approccio modellistico che consenta la valutazione dell’impatto idrologico del cambiamento climatico su due bacini del Mediterraneo localizzati in Sardegna. Questo contributo si focalizza su due temi principali: capire come la rappresentazione fisica dei modelli idrologici incida sulla valutazione dell’impatto idrologico dovuto al cambiamento climatico su un bacino con un clima semi-arido, il Rio Mannu di San Sperate, e dimostrare come la modellizzazione avanzata possa aiutare nel definire misure di adattamento in un sistema idrico complesso incline ad eventi estremi, il Flumendosa, in condizioni di cambiamento climatico. Per raggiungere tale obiettivo il lavoro si articola in tre fasi. Gli effetti del cambiamento climatico sul bacino del Rio Mannu sono stati valutati attraverso il confronto dei risultati di cinque modelli idrologici, CATchment HYdrology (CATHY), Soil and Water Assessment Tool (SWAT), TIN-based Real time Integrated Basin Simulator (tRIBS), TOPographic Kinematic APproximation and Integration-eXtended (TOPKAPI-X), and Water flow and balance Simulation Model (WASIM), utilizzando come forzante atmosferica gli output di quattro combinazioni di modelli climatici globali (GCM) e regionali (RCM). Per valutare le incertezze è stata utilizzata una metrica recentemente proposta: i risultati dei modelli sono stati comparati durante un periodo di riferimento e futuro, utilizzando l’indice di correlazione di Pearson e il bias di Duveiller. Pur con qualche differenza, complessivamente i modelli idrologici mostrano una buona concordanza tra loro, e rispondono in maniera simile alla riduzione della precipitazione e all’incremento della temperatura previsti dai modelli climatici. Ci si aspetta pertanto che il bacino nel futuro sarà soggetto ad una riduzione della disponibilità di risorsa idrica, con conseguenze negative in particolare per il settore agricolo. È stato effettuato un confronto dettagliato delle risposte ottenute sullo stesso bacino con tre modelli idrologici fisicamente basati di diverso grado per quanto riguarda la rappresentazione dei processi fisici e delle caratteristiche del terreno, CATHY, TOPKAPI-X, tRIBS, con lo scopo di testare la trasferibilità dei parametri tra i tre modelli idrologici, concentrandosi sulle difficoltà riscontrate nei periodi di calibrazione e validazione. Mentre i tre modelli hanno risposto in maniera simile durante il periodo di calibrazione, sono state riscontrate significative differenze durante il periodo di validazione, caratterizzato da un clima molto secco, con il modello CATHY, che ha prodotto una portata molto bassa. Pertanto, per ottenere risultati soddisfacenti con il modello CATHY, è stata assunta l’ipotesi di soil crusting, sulla base della quale il primo strato di suolo è stato modellato con una ridotta conducibilità idraulica satura. Infine il modello TOPKAPI-X è stato implementato su uno dei principali bacini sardi di importanza strategica per il sistema idrico della regione, il Flumendosa, per valutare gli effetti del cambiamento climatico a scala maggiore. Il modello risponde con una diminuzione dei valori di portata, contenuto idrico ed evapotraspirazione reale alla riduzione della precipitazione ed incremento della temperature previsto dai modelli climatici, dando supporto ad uno scenario futuro di carenza della risorsa idrica anche in questo bacino dell’area Mediterranea.

This study aims to evaluate the effects of the Canadian Regional Climate Model’s (CRCM) spatial resolution on summer-fall floods simulation. Seven different climate simulations issued from the fourth and the fifth version of the CRCM are employed. Four different climate simulations issued from the fourth version of the CRCM (CRCM4) are compared. They are composed of two simulations driven by the Canadian General Circulation Model (CGCM) and two driven by the ERA-40c reanalysis using grid meshes of 15 km and 45 km resolutions for each driver. Three climate simulations issued from the fifth version of the CRCM (CRCM5) driven by the ERA-Interim at 0.44° (≈ 48 km), 0.22° (≈ 24 km) and 0.11° (≈ 12 km) spatial resolutions are used. All comparisons are evaluated on a daily time-step for the 1961-1990 period (for CRCM4) and for the 1981-2010 period (for CRCM5). These seven simulations (four from CRCM4 and three from CRCM5) are used as input for two hydrological models of varying complexity (HSAMI and MOHYSE). Each model is calibrated using three different objective functions based on the Kling-Gupta Efficiency criteria (KGE) to target the summer-fall floods. Three seasonal indices are used to evaluate the CRCM outputs: bias (temperature), relative bias (precipitation) and variances ratio (temperature and precipitation). In an attempt to evaluate the effects of the spatial resolution on the hydrological modelling of summer-fall floods, streamflow simulations are generated using the seven climate datasets. The generated climate-driven streamflow simulations are analysed by two performance statistics: the seasonal values of KGE and the seasonal relative biases. Summer-fall floods are evaluated through the use of four flood indicators, the 2-year, 5-year, 10-year and 20-year return periods. The results revealed an impact of spatial resolution on climate model outputs (temperature and precipitation) and on summer-fall floods simulation by the two hydrological models and the three different calibration approaches, although this can be due to other elements such as domain size and climate model driver. The flood indicators demonstrate an increase on the summer-fall floods return periods with increasing resolution from both hydrological models. On the other hand the hydrological models structure and the calibration approaches did not show significant impacts on the summer-fall floods. The results highlight the need for further research to assess the additional uncertainty due to the impacts of the climate simulations spatial resolution on hydrological studies.

With the growing realization that crystallization processes may evolve through a sequence of different solid forms, including amorphous precursor phases, the development of suitable in-situ experimental probes is essential for comprehensively mapping the time-evolution of such processes. Here we demonstrate that the CLASSIC NMR (Combined Liquid- And Solid-State In-situ Crystallization NMR) strategy is a powerful technique for revealing the transitory existence of amorphous phases during crystallization processes, applying this technique to study crystallization of dl-menthol and l-menthol from their molten liquid phases. The CLASSIC NMR results provide direct insights into the conditions (including the specific time period) under which the molten liquid phase, transitory amorphous phases and final crystalline phases exist during these crystallization processes.

Evaluating the historical contribution of the volume loss of ice to stream flow based on reconstructed volume changes through the Little Ice Age (LIA) can be directly related to the understanding of glacier-hydrology in the current epoch of rapid glacier loss that has disquieting implications for a water resource in the Cordillera Blanca in the Peruvian Andes. However, the accurate prediction of the future glacial meltwater availability for the developing regional Andean society needs more extensive quantitative estimation from long-term glacial meltwater of reconstructed glacial volume. Modeling the LIA paleoglaciers through the mid-19th century (with the most extensive recent period of mountain glacier expansion having occurred around 1850 AD) in different catchments of the Cordillera Blanca allows us to reconstruct glacier volume and its change from likely combinations of climatic control variables and time. We computed the rate and magnitude of centennial-scale glacier volume changes for glacier surfaces between the LIA and the modern era, as defined by 2011 Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) Global Digital Elevation Model Version 2 (GDEM V2) and 2008 Light Detection and Range (LiDAR) data. The model simulation showed good agreement with the observed geomorphic data and the volume and surface area (V-S) scaling remained within the 25% error range in the reconstructed simulation. Also, we employed a recently demonstrated approach (Baraër, M. et al.) to calculate meltwater contribution to glacierized catchment runoff. The results revealed multiple peaks of both mean annual and dry season discharge that have never been shown in previous research on the same mountain range.

The rapidly melting glaciers of Peru are posing new risks to regional dry season water supplies, and this is evident in the Cordillera Blanca, the mountain range with the world's largest concentration of tropical glaciers. Permanent ice loss is causing reductions to dry season streamflow, which is coupled with shifting demands and control over water access and entitlements in the region. A full evaluation of hydrologic inputs is required to inform future water management in the relative absence of glaciers. Over the last decade, new studies have shown groundwater to be a significant component of the regional water budget during the dry season, and it cannot be ignored when accounting for water quality and quantity downstream of the Cordillera Blanca's alpine catchments. Distinctive common features of the Cordillera Blanca's proglacial catchments are sediment‐filled valleys that were once under proglacial lake conditions. The combination of lake sediments with other alpine depositional features results in storage and interseasonal release of groundwater that comprises up to 80% of the valley's streamflow during the driest months of the year. We summarize the emerging understanding of hydrogeologic processes in proglacial headwater systems of the region's principal river, the Rio Santa, and make suggestions for future research that will more clearly characterize the spatial distribution of stored groundwater within the mountain range. As glaciers continue to recede, differences in aquifer thickness and groundwater residence time between alpine catchments in the region will increasingly control dry season water availability at the local and basin scale. This article is categorized under: Science of Water > Hydrological Processes Science of Water > Water and Environmental Change Engineering Water > Planning Water

Abstract. Black carbon aerosol (BC), which is emitted from natural and anthropogenic sources (e.g., wildfires, coal burning), can contribute to magnify climate warming at high latitudes by darkening snow- and ice-covered surfaces, and subsequently lowering their albedo. Therefore, modeling the atmospheric transport and deposition of BC to the Arctic is important, and historical archives of BC accumulation in polar ice can help to validate such modeling efforts. Here we present a > 250-year ice-core record of refractory BC (rBC) deposition on Devon ice cap, Canada, spanning the years from 1735 to 1992. This is the first such record ever developed from the Canadian Arctic. The estimated mean deposition flux of rBC on Devon ice cap for 1963–1990 is 0.2 mg m−2 a−1, which is at the low end of estimates from Greenland ice cores obtained using the same analytical method ( ∼ 0.1–4 mg m−2 a−1). The Devon ice cap rBC record also differs from the Greenland records in that it shows only a modest increase in rBC deposition during the 20th century. In the Greenland records a pronounced rise in rBC is observed from the 1880s to the 1910s, which is largely attributed to midlatitude coal burning emissions. The deposition of contaminants such as sulfate and lead increased on Devon ice cap in the 20th century but no concomitant rise in rBC is recorded in the ice. Part of the difference with Greenland could be due to local factors such as melt–freeze cycles on Devon ice cap that may limit the detection sensitivity of rBC analyses in melt-impacted core samples, and wind scouring of winter snow at the coring site. Air back-trajectory analyses also suggest that Devon ice cap receives BC from more distant North American and Eurasian sources than Greenland, and aerosol mixing and removal during long-range transport over the Arctic Ocean likely masks some of the specific BC source–receptor relationships. Findings from this study suggest that there could be a large variability in BC aerosol deposition across the Arctic region arising from different transport patterns. This variability needs to be accounted for when estimating the large-scale albedo lowering effect of BC deposition on Arctic snow/ice.