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Abstract. The Last Glacial Maximum (LGM; 21 000 yr before present) was a period of low atmospheric greenhouse gas concentrations, when vast ice sheets covered large parts of North America and Europe. Paleoclimate reconstructions and modeling studies suggest that the atmospheric circulation was substantially altered compared to today, both in terms of its mean state and its variability. Here we present a suite of coupled model simulations designed to investigate both the separate and combined influences of the main LGM boundary condition changes (greenhouse gases, ice sheet topography and ice sheet albedo) on the mean state and variability of the atmospheric circulation as represented by sea level pressure (SLP) and 200-hPa zonal wind in the North Atlantic sector. We find that ice sheet topography accounts for most of the simulated changes during the LGM. Greenhouse gases and ice sheet albedo affect the SLP gradient in the North Atlantic, but the overall placement of high and low pressure centers is controlled by topography. Additional analysis shows that North Atlantic sea surface temperatures and sea ice edge position do not substantially influence the pattern of the climatological-mean SLP field, SLP variability or the position of the North Atlantic jet in the LGM.

Abstract. Ozone pollution represents a serious health and environmental problem. While ozone pollution is mostly produced by photochemistry in summer, elevated ozone concentrations can also be influenced by long range transport driven by the atmospheric circulation and stratospheric ozone intrusions. We analyze the role of large scale atmospheric circulation variability in the North Atlantic basin in determining surface ozone concentrations over Europe. Here, we show, using ground station measurements and a coupled atmosphere-chemistry model simulation for the period 1980–2005, that the North Atlantic Oscillation (NAO) does affect surface ozone concentrations – on a monthly timescale, over 10 ppbv in southwestern, central and northern Europe – during all seasons except fall. The commonly used NAO index is able to capture the link existing between atmospheric dynamics and surface ozone concentrations in winter and spring but it fails in summer. We find that the first Principal Component, computed from the time variation of the sea level pressure (SLP) field, detects the atmosphere circulation/ozone relationship not only in winter and spring but also during summer, when the atmospheric circulation weakens and regional photochemical processes peak. Given the NAO forecasting skill at intraseasonal time scale, the first Principal Component of the SLP field could be used as an indicator to identify areas more exposed to forthcoming ozone pollution events. Finally, our results suggest that the increasing baseline ozone in western and northern Europe during the 1990s could be related to the prevailing positive phase of the NAO in that period.

In this study we use a global climate model to assess particulate matter (PM) variability induced by the North Atlantic Oscillation (NAO) in Europe during winter and the potential impact on human health of a future shift in the NAO mean state. Our study shows that extreme NAO phases in the 1990s modulated most of the interannual variability of winter PM concentrations in several European countries. Increased PM concentrations as a result of a positive shift in the mean winter NAO of one standard deviation would lead to about 5500 additional premature deaths in Mediterranean countries, compared to the simulated average PM health impact for the year 2000. In central‐northern Europe, instead, higher wind speed and increased PM removal by precipitation lead to negative PM concentration anomalies with associated health benefits. We suggest that the NAO index is a useful indicator for the role of interannual atmospheric variability on large‐scale pollution‐health impacts. , Key Points NAO impacts on PM concentrations Potential impacts of NAO shifts on human health Large‐scale atmospheric indicators as proxy for risk estimates of PM episodes

Abstract. Numerical model scenarios of future climate depict a global increase in temperatures and changing precipitation patterns, primarily driven by increasing greenhouse gas (GHG) concentrations. Aerosol particles also play an important role by altering the Earth's radiation budget and consequently surface temperature. Here, we use the general circulation aerosol model ECHAM5-HAM, coupled to a mixed layer ocean model, to investigate the impacts of future air pollution mitigation strategies in Europe on winter atmospheric circulation over the North Atlantic. We analyse the extreme case of a maximum feasible end-of-pipe reduction of aerosols in the near future (2030), in combination with increasing GHG concentrations. Our results show a more positive North Atlantic Oscillation (NAO) mean state by 2030, together with a significant eastward shift of the southern centre of action of sea-level pressure (SLP). Moreover, we show a significantly increased blocking frequency over the western Mediterranean. By separating the impacts of aerosols and GHGs, our study suggests that future aerosol abatement may be the primary driver of both the eastward shift in the southern SLP centre of action and the increased blocking frequency over the western Mediterranean. These concomitant modifications of the atmospheric circulation over the Euro-Atlantic sector lead to more stagnant weather conditions that favour air pollutant accumulation, especially in the western Mediterranean sector. Changes in atmospheric circulation should therefore be included in future air pollution mitigation assessments. The indicator-based evaluation of atmospheric circulation changes presented in this work will allow an objective first-order assessment of the role of changes in wintertime circulation on future air quality in other climate model simulations.

Abstract. Reconstructions of Quaternary climate are often based on the isotopic content of paleo-precipitation preserved in proxy records. While many paleo-precipitation isotope records are available, few studies have synthesized these dispersed records to explore spatial patterns of late-glacial precipitation δ18O. Here we present a synthesis of 86 globally distributed groundwater (n = 59), cave calcite (n = 15) and ice core (n = 12) isotope records spanning the late-glacial (defined as ~ 50 000 to ~ 20 000 years ago) to the late-Holocene (within the past ~ 5000 years). We show that precipitation δ18O changes from the late-glacial to the late-Holocene range from −7.1 ‰ (δ18Olate-Holocene > δ18Olate-glacial) to +1.7 ‰ (δ18Olate-glacial > δ18Olate-Holocene), with the majority (77 %) of records having lower late-glacial δ18O than late-Holocene δ18O values. High-magnitude, negative precipitation δ18O shifts are common at high latitudes, high altitudes and continental interiors (δ18Olate-Holocene > δ18Olate-glacial by more than 3 ‰). Conversely, low-magnitude, positive precipitation δ18O shifts are concentrated along tropical and subtropical coasts (δ18Olate-glacial > δ18Olate-Holocene by less than 2 ‰). Broad, global patterns of late-glacial to late-Holocene precipitation δ18O shifts suggest that stronger-than-modern isotopic distillation of air masses prevailed during the late-glacial, likely impacted by larger global temperature differences between the tropics and the poles. Further, to test how well general circulation models reproduce global precipitation δ18O shifts, we compiled simulated precipitation δ18O shifts from five isotope-enabled general circulation models simulated under recent and last glacial maximum climate states. Climate simulations generally show better inter-model and model-measurement agreement in temperate regions than in the tropics, highlighting a need for further research to better understand how inter-model spread in convective rainout, seawater δ18O and glacial topography parameterizations impact simulated precipitation δ18O. Future research on paleo-precipitation δ18O records can use the global maps of measured and simulated late-glacial precipitation isotope compositions to target and prioritize field sites.

Significance In the model simulations analyzed here, large high-latitude volcanic eruptions have global and long-lasting effects on climate, altering the spatiotemporal characteristic of the El Niño–Southern Oscillation (ENSO) on both short (<1 y) and long timescales and affecting the strength of the Atlantic Meridional Overturning Circulation (AMOC). In the first 8–9 mo following the start of the eruption, El Niño-like anomalies develop over the equatorial Pacific. The large high-latitude eruptions also trigger a strengthening of the AMOC in the first 25 y after the eruption, which is associated with an increase in ENSO variability. This is then followed by a weakening of the AMOC lasting another 30–35 y, associated with decreased ENSO variability. , Large volcanic eruptions can have major impacts on global climate, affecting both atmospheric and ocean circulation through changes in atmospheric chemical composition and optical properties. The residence time of volcanic aerosol from strong eruptions is roughly 2–3 y. Attention has consequently focused on their short-term impacts, whereas the long-term, ocean-mediated response has not been well studied. Most studies have focused on tropical eruptions; high-latitude eruptions have drawn less attention because their impacts are thought to be merely hemispheric rather than global. No study to date has investigated the long-term effects of high-latitude eruptions. Here, we use a climate model to show that large summer high-latitude eruptions in the Northern Hemisphere cause strong hemispheric cooling, which could induce an El Niño-like anomaly, in the equatorial Pacific during the first 8–9 mo after the start of the eruption. The hemispherically asymmetric cooling shifts the Intertropical Convergence Zone southward, triggering a weakening of the trade winds over the western and central equatorial Pacific that favors the development of an El Niño-like anomaly. In the model used here, the specified high-latitude eruption also leads to a strengthening of the Atlantic Meridional Overturning Circulation (AMOC) in the first 25 y after the eruption, followed by a weakening lasting at least 35 y. The long-lived changes in the AMOC strength also alter the variability of the El Niño–Southern Oscillation (ENSO).

Abstract Sources and timing of freshwater forcing relative to hydroclimate shifts recorded in Greenland ice cores at the onset of Younger Dryas, ∼12,800 years ago, remain speculative. Here we show that progressive Fennoscandian Ice Sheet (FIS) melting 13,100–12,880 years ago generates a hydroclimate dipole with drier–colder conditions in Northern Europe and wetter–warmer conditions in Greenland. FIS melting culminates 12,880 years ago synchronously with the start of Greenland Stadial 1 and a large-scale hydroclimate transition lasting ∼180 years. Transient climate model simulations forced with FIS freshwater reproduce the initial hydroclimate dipole through sea-ice feedbacks in the Nordic Seas. The transition is attributed to the export of excess sea ice to the subpolar North Atlantic and a subsequent southward shift of the westerly winds. We suggest that North Atlantic hydroclimate sensitivity to FIS freshwater can explain the pace and sign of shifts recorded in Greenland at the climate transition into the Younger Dryas.

Abstract The last deglaciation (20.0–10.0 kyr B.P.) was punctuated by two major cooling events affecting the Northern Hemisphere: the Oldest Dryas (OD; 18.0–14.7 kyr B.P.) and the Younger Dryas (YD; 12.8–11.5 kyr B.P.). Greenland ice core δ 18 O temperature reconstructions suggest that the YD was as cold as the OD, despite a 50 ppmv increase in atmospheric CO 2 , while modeling studies suggest that the YD was approximately 4–5°C warmer than the OD. This discrepancy has been surmised to result from changes in the origin of the water vapor delivered to Greenland; however, this hypothesis has not been hitherto tested. Here we use an atmospheric circulation model with an embedded moisture‐tracing module to investigate atmospheric processes that may have been responsible for the similar δ 18 O values during the OD and YD. Our results show that the summer‐to‐winter precipitation ratio over central Greenland in the OD is twice as high as in the YD experiment, which shifts the δ 18 O signal toward warmer (summer) temperatures (enriched δ 18 O values and it accounts for ~45% of the expected YD‐OD δ 18 O difference). A change in the inversion (cloud) temperature relationship between the two climate states further contributes (~20%) to altering the δ 18 O‐temperature‐relation model. Our experiments also show a 7% decrease of δ 18 O‐depleted precipitation from distant regions (e.g., the Pacific Ocean) in the OD, hence further contributing (15–20%) in masking the actual temperature difference. All together, these changes provide a physical explanation for the ostensible similarity in the ice core δ 18 O temperature reconstructions in Greenland during OD and YD. , Key Points Precipitation seasonality and inversion temperature changes behind YD‐OD δ 18 O enigma Local processes changes accounting up to 65% of the expected YD‐OD δ 18 O difference Moisture transport changes from the Pacific accounting only up to 20% of the expected YD‐OD δ 18 O difference

Abstract The summer rainfall across Sahelian‐Sudan is one of the main sources of water for agriculture, human, and animal needs. However, the rainfall is characterized by large interannual variability, which has attracted extensive scientific efforts to understand it. This study attempts to identify the source regions that contribute to the Sahelian‐Sudan moisture budget during July through September. We have used an atmospheric general circulation model with an embedded moisture‐tracing module (Community Atmosphere Model version 3), forced by observed (1979–2013) sea‐surface temperatures. The result suggests that about 40% of the moisture comes with the moisture flow associated with the seasonal migration of the Intertropical Convergence Zone (ITCZ) and originates from Guinea Coast, central Africa, and the Western Sahel. The Mediterranean Sea, Arabian Peninsula, and South Indian Ocean regions account for 10.2%, 8.1%, and 6.4%, respectively. Local evaporation and the rest of the globe supply the region with 20.3% and 13.2%, respectively. We also compared the result from this study to a previous analysis that used the Lagrangian model FLEXPART forced by ERA‐Interim. The two approaches differ when comparing individual regions, but are in better agreement when neighboring regions of similar atmospheric flow features are grouped together. Interannual variability with the rainfall over the region is highly correlated with contributions from regions that are associated with the ITCZ movement, which is in turn linked to the Atlantic Multidecadal Oscillation. Our result is expected to provide insights for the effort on seasonal forecasting of the rainy season over Sahelian Sudan. , Key Points The moisture associated with ITCZ flow accounts for about 40%‐50% of the precipitated water The local evaporation provides about 20% of the precipitated water The multiyear variability in the rainfall seems to be linked to the AMO

Abstract A large ensemble of Earth System Model simulations is analyzed to show that high‐latitude Northern Hemisphere eruptions give rise to El Niño‐like anomalies in the winter following the eruption, the amplitude of which depends on the state of the tropical Pacific at the time of the eruption. The El Niño‐like anomalies are almost three times larger when the eruption occurs during an incipient La Niña or during a neutral state compared to an incipient El Niño. The differential response results from stronger atmosphere‐ocean coupling and extra‐tropical feedbacks during an incipient La Niña compared to El Niño. Differences in the response continue through the second and third years following the eruption. When the eruption happens in a year of an incipient El Niño, a large cold (La Niña‐like) anomaly develops in year 2; if the eruption occurs in a year of an incipient La Niña, no anomalies are simulated in year 2 and a La Niña‐like response appears in year 3. After the El Niño‐like anomaly in the first winter, the overall tendency of ENSO in the following 2 years is toward a La Niña state. Our results highlight the high sensitivity of tropical Pacific dynamics under volcanic forcing to the ENSO initial state and lay the groundwork for improved predictions of the global climatic response to high‐latitude volcanic eruptions. , Key Points HL eruptions alter the mean state of ENSO, and detectable anomalies are seen up to 3 years after the eruption Stronger El Niño‐like anomalies on year 1 when eruptions occurs under developing La Niñas La Niña‐like anomalies on year 2 and year 3 when eruptions occurs under developing El Niños and La Niñas, respectively

Abstract. The enhancement of the stratospheric aerosol layer by volcanic eruptions induces a complex set of responses causing global and regional climate effects on a broad range of timescales. Uncertainties exist regarding the climatic response to strong volcanic forcing identified in coupled climate simulations that contributed to the fifth phase of the Coupled Model Intercomparison Project (CMIP5). In order to better understand the sources of these model diversities, the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP) has defined a coordinated set of idealized volcanic perturbation experiments to be carried out in alignment with the CMIP6 protocol. VolMIP provides a common stratospheric aerosol data set for each experiment to minimize differences in the applied volcanic forcing. It defines a set of initial conditions to assess how internal climate variability contributes to determining the response. VolMIP will assess to what extent volcanically forced responses of the coupled ocean–atmosphere system are robustly simulated by state-of-the-art coupled climate models and identify the causes that limit robust simulated behavior, especially differences in the treatment of physical processes. This paper illustrates the design of the idealized volcanic perturbation experiments in the VolMIP protocol and describes the common aerosol forcing input data sets to be used.

Abstract Here, we use a coupled atmospheric‐ocean‐aerosol model to investigate the plume development and climate effects of the smoke generated by fires following a regional nuclear war between emerging third‐world nuclear powers. We simulate a standard scenario where 5 Tg of black carbon ( BC ) is emitted over 1 day in the upper troposphere–lower stratosphere. However, it is likely that the emissions from the fires ignited by bomb detonations include a substantial amount of particulate organic matter ( POM ) and that they last more than 1 day. We therefore test the sensitivity of the aerosol plume and climate system to the BC / POM ratio (1:3, 1:9) and to the emission length (1 day, 1 week, 1 month). We find that in general, an emission length of 1 month substantially reduces the cooling compared to the 1‐day case, whereas taking into account POM emissions notably increases the cooling and the reduction of precipitation associated with the nuclear war during the first year following the detonation. Accounting for POM emissions increases the particle size in the short‐emission‐length scenarios (1 day/1 week), reducing the residence time of the injected particle. While the initial cooling is more intense when including POM emission, the long‐lasting effects, while still large, may be less extreme compared to the BC ‐only case. Our study highlights that the emission altitude reached by the plume is sensitive to both the particle type emitted by the fires and the emission duration. Consequently, the climate effects of a nuclear war are strongly dependent on these parameters. , Key Points Importance of including OC when simulating nuclear wars Importance of the fire emission length when simulating nuclear wars

We estimate rainfall during the “Green Sahara” period. , During the “Green Sahara” period (11,000 to 5000 years before the present), the Sahara desert received high amounts of rainfall, supporting diverse vegetation, permanent lakes, and human populations. Our knowledge of rainfall rates and the spatiotemporal extent of wet conditions has suffered from a lack of continuous sedimentary records. We present a quantitative reconstruction of western Saharan precipitation derived from leaf wax isotopes in marine sediments. Our data indicate that the Green Sahara extended to 31°N and likely ended abruptly. We find evidence for a prolonged “pause” in Green Sahara conditions 8000 years ago, coincident with a temporary abandonment of occupational sites by Neolithic humans. The rainfall rates inferred from our data are best explained by strong vegetation and dust feedbacks; without these mechanisms, climate models systematically fail to reproduce the Green Sahara. This study suggests that accurate simulations of future climate change in the Sahara and Sahel will require improvements in our ability to simulate vegetation and dust feedbacks.

Abstract A generalized linear model based on Poisson regression has been used to assess the impact of environmental variables modulating tropical cyclone frequency in six main cyclone development areas: the East Pacific, West Pacific, North Atlantic, North Indian, South Indian, and South Pacific. The analysis covers the period 1980–2009 and focuses on widely used meteorological parameters including wind shear, sea surface temperature, and relative humidity from different reanalyses as well as aerosol optical depth for different compounds simulated by the Goddard Chemistry Aerosol Radiation and Transport model. Circulation indices are also included. Cyclone frequency is obtained from the International Best Track Archive for Climate Stewardship. A strong link is found between cyclone frequency and the relative sea surface temperature, Atlantic Meridional Mode, and wind shear with significant explained log likelihoods in the North Atlantic of 37%, 27%, and 28%, respectively. A significant impact of black carbon and organic aerosols on cyclone frequency is found over the North Indian Ocean, with explained log likelihoods of 27%. A weaker but still significant impact is found for observed dust aerosols in the North Atlantic with an explained log likelihood of 11%. Changes in lower stratospheric temperatures explain 28% of the log likelihood in the North Atlantic. Lower stratospheric temperatures from a subset of Coupled Model Intercomparison Project Phase 5 models properly simulate the warming and subsequent cooling of the lower stratosphere that follows a volcanic eruption but underestimates the cooling by about 0.5°C. , Key Points Significant impact of black carbon and organic aerosols Significant impact of observed dust aerosols in the North Atlantic Lower stratospheric temperatures explain 28% of the log likelihood

Abstract Experiments with a climate model (NorESM1) were performed to isolate the effects of aerosol particles and greenhouse gases on surface temperature and precipitation in simulations of future climate. The simulations show that by 2025–49 a reduction of aerosol emissions from fossil fuels following a maximum technically feasible reduction (MFR) scenario could lead to a global and Arctic warming of 0.26 and 0.84 K, respectively, as compared with a simulation with fixed aerosol emissions at the level of 2005. If fossil fuel emissions of aerosols follow a current legislation emissions (CLE) scenario, the NorESM1 model simulations yield a nonsignificant change in global and Arctic average surface temperature as compared with aerosol emissions fixed at year 2005. The corresponding greenhouse gas effect following the representative concentration pathway 4.5 (RCP4.5) emission scenario leads to a global and Arctic warming of 0.35 and 0.94 K, respectively. The model yields a marked annual average northward shift in the intertropical convergence zone with decreasing aerosol emissions and subsequent warming of the Northern Hemisphere. The shift is most pronounced in the MFR scenario but also visible in the CLE scenario. The modeled temperature response to a change in greenhouse gas concentrations is relatively symmetric between the hemispheres, and there is no marked shift in the annual average position of the intertropical convergence zone. The strong reduction in aerosol emissions in the MFR scenario also leads to a net southward cross-hemispheric energy transport anomaly both in the atmosphere and ocean, and enhanced monsoon circulation in Southeast Asia and East Asia causing an increase in precipitation over a large part of this region.

Significance Our modeling study shows the crucial role of vegetation cover over the Sahara and reduced dust emission in altering tropical cyclone activity during the mid-Holocene (6,000 yBP). Our results also demonstrate how these regional changes in land cover and dust emission are able to affect areas far afield through changes of large-scale atmospheric circulation. Our study strongly suggests that an appropriate representation of land cover and dust emission is of paramount importance to be able to capture past—and potentially future—climate changes. , Tropical cyclones (TCs) can have devastating socioeconomic impacts. Understanding the nature and causes of their variability is of paramount importance for society. However, historical records of TCs are too short to fully characterize such changes and paleo-sediment archives of Holocene TC activity are temporally and geographically sparse. Thus, it is of interest to apply physical modeling to understanding TC variability under different climate conditions. Here we investigate global TC activity during a warm climate state (mid-Holocene, 6,000 yBP) characterized by increased boreal summer insolation, a vegetated Sahara, and reduced dust emissions. We analyze a set of sensitivity experiments in which not only solar insolation changes are varied but also vegetation and dust concentrations. Our results show that the greening of the Sahara and reduced dust loadings lead to more favorable conditions for tropical cyclone development compared with the orbital forcing alone. In particular, the strengthening of the West African Monsoon induced by the Sahara greening triggers a change in atmospheric circulation that affects the entire tropics. Furthermore, whereas previous studies suggest lower TC activity despite stronger summer insolation and warmer sea surface temperature in the Northern Hemisphere, accounting for the Sahara greening and reduced dust concentrations leads instead to an increase of TC activity in both hemispheres, particularly over the Caribbean basin and East Coast of North America. Our study highlights the importance of regional changes in land cover and dust concentrations in affecting the potential intensity and genesis of past TCs and suggests that both factors may have appreciable influence on TC activity in a future warmer climate.

Abstract The Caribbean low‐level jet (CLLJ) is an important modulator of regional climate, especially precipitation, in the Caribbean and Central America. Previous work has inferred, due to their semiannual cycle, an association between CLLJ strength and meridional sea surface temperature (SST) gradients in the Caribbean Sea, suggesting that the SST gradients may control the intensity and vertical shear of the CLLJ. In addition, both the horizontal and vertical structure of the jet have been related to topographic effects via interaction with the mountains in Northern South America (NSA), including funneling effects and changes in the meridional geopotential gradient. Here we test these hypotheses, using an atmospheric general circulation model to perform a set of sensitivity experiments to examine the impact of both SST gradients and topography on the CLLJ. In one sensitivity experiment, we remove the meridional SST gradient over the Caribbean Sea and in the other, we flatten the mountains over NSA. Our results show that the SST gradient and topography have little or no impact on the jet intensity, vertical, and horizontal wind shears, contrary to previous works. However, our findings do not discount a possible one‐way coupling between the SST and the wind over the Caribbean Sea through friction force. We also examined an alternative approach based on barotropic instability to understand the CLLJ intensity, vertical, and horizontal wind shears. Our results show that the current hypothesis about the CLLJ must be reviewed in order to fully understand the atmospheric dynamics governing the Caribbean region. , Key Points Atmospheric dynamics in the Caribbean SST over the Caribbean Sea is examined as kinetic energy source for the CLLJ Impact of meridional SST gradient on the vertical structure of CLLJ

Abstract Understanding the West African monsoon (WAM) dynamics in the mid-Holocene (MH) is a crucial issue in climate modeling, because numerical models typically fail to reproduce the extensive precipitation suggested by proxy evidence. This discrepancy may be largely due to the assumption of both unrealistic land surface cover and atmospheric aerosol concentration. In this study, the MH environment is simulated in numerical experiments by imposing extensive vegetation over the Sahara and the consequent reduction in airborne dust concentration. A dramatic increase in precipitation is simulated across the whole of West Africa, up to the Mediterranean coast. This precipitation response is in better agreement with proxy data, in comparison with the case in which only changes in orbital forcing are considered. Results show a substantial modification of the monsoonal circulation, characterized by an intensification of large-scale deep convection through the entire Sahara, and a weakening and northward shift (~6.5°) of the African easterly jet. The greening of the Sahara also leads to a substantial reduction in the African easterly wave activity and associated precipitation. The reorganization of the regional atmospheric circulation is driven by the vegetation effect on radiative forcing and associated heat fluxes, with the reduction in dust concentration to enhance this response. The results for the WAM in the MH present important implications for understanding future climate scenarios in the region and in teleconnected areas, in the context of projected wetter conditions in West Africa.