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Polar clouds are, as a consequence of the paucity of in situ observations, poorly understood compared to their lower latitude analogs, yet highly climate-sensitive through thermal radiation emission. The prevalence of Thin Ice Clouds (TIC) dominates in cold Polar Regions and the Upper Troposphere Lower Stratosphere (UTLS) altitudes. They can be grouped into 2 broad categories. The first thin ice cloud type (TIC1) is made up of high concentrations of small, non-precipitating ice crystals. The second type (TIC2) is composed of relatively small concentrations of larger, precipitating ice crystals. In this study, we investigate the ability of a developmental version of the Canadian Regional Climate Model (CRCM6) in simulating cold polar-night clouds over the Arctic Ocean, a remote region that is critical to atmospheric circulation reaching out to the mid-latitudes. The results show that, relative to CloudSat-CALIPSO vertical profile products, CRCM6 simulates high-latitude and low spatial frequency variations of Ice Water Content (IWC), effective radius (re) and cooling rates reasonably well with only small to moderate wet and dry biases. The model can also simulate cloud type, location, and temporal occurrence effectively. As well, it successfully simulated higher altitude TIC1 clouds whose small size evaded CloudSat detection while being visible to CALIPSO.
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Abstract. Starphotometry, the night-time counterpart of sunphotometry, has not yet achieved the commonly sought observational error level of 1 %: a spectral optical depth (OD) error level of 0.01. In order to address this issue, we investigate a large variety of systematic (absolute) uncertainty sources. The bright-star catalogue of extraterrestrial references is noted as a major source of errors with an attendant recommendation that its accuracy, particularly its spectral photometric variability, be significantly improved. The small field of view (FOV) employed in starphotometry ensures that it, unlike sun- or moonphotometry, is only weakly dependent on the intrinsic and artificial OD reduction induced by scattering into the FOV by optically thin clouds. A FOV of 45 arcsec (arcseconds) was found to be the best trade-off for minimizing such forward-scattering errors concurrently with flux loss through vignetting. The importance of monitoring the sky background and using interpolation techniques to avoid spikes and to compensate for measurement delay was underscored. A set of 20 channels was identified to mitigate contamination errors associated with stellar and terrestrial atmospheric gas absorptions, as well as aurora and airglow emissions. We also note that observations made with starphotometers similar to our High Arctic instrument should be made at high angular elevations (i.e. at air masses less than 5). We noted the significant effects of snow crystal deposition on the starphotometer optics, how pseudo OD increases associated with this type of contamination could be detected, and how proactive techniques could be employed to avoid their occurrence in the first place. If all of these recommendations are followed, one may aspire to achieve component errors that are well below 0.01: in the process, one may attain a total 0.01 OD target error.
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Abstract. Motivated by the need to predict how the Arctic atmosphere will change in a warming world, this article summarizes recent advances made by the research consortium NETCARE (Network on Climate and Aerosols: Addressing Key Uncertainties in Remote Canadian Environments) that contribute to our fundamental understanding of Arctic aerosol particles as they relate to climate forcing. The overall goal of NETCARE research has been to use an interdisciplinary approach encompassing extensive field observations and a range of chemical transport, earth system, and biogeochemical models. Several major findings and advances have emerged from NETCARE since its formation in 2013. (1) Unexpectedly high summertime dimethyl sulfide (DMS) levels were identified in ocean water (up to 75 nM) and the overlying atmosphere (up to 1 ppbv) in the Canadian Arctic Archipelago (CAA). Furthermore, melt ponds, which are widely prevalent, were identified as an important DMS source (with DMS concentrations of up to 6 nM and a potential contribution to atmospheric DMS of 20 % in the study area). (2) Evidence of widespread particle nucleation and growth in the marine boundary layer was found in the CAA in the summertime, with these events observed on 41 % of days in a 2016 cruise. As well, at Alert, Nunavut, particles that are newly formed and grown under conditions of minimal anthropogenic influence during the months of July and August are estimated to contribute 20 % to 80 % of the 30–50 nm particle number density. DMS-oxidation-driven nucleation is facilitated by the presence of atmospheric ammonia arising from seabird-colony emissions, and potentially also from coastal regions, tundra, and biomass burning. Via accumulation of secondary organic aerosol (SOA), a significant fraction of the new particles grow to sizes that are active in cloud droplet formation. Although the gaseous precursors to Arctic marine SOA remain poorly defined, the measured levels of common continental SOA precursors (isoprene and monoterpenes) were low, whereas elevated mixing ratios of oxygenated volatile organic compounds (OVOCs) were inferred to arise via processes involving the sea surface microlayer. (3) The variability in the vertical distribution of black carbon (BC) under both springtime Arctic haze and more pristine summertime aerosol conditions was observed. Measured particle size distributions and mixing states were used to constrain, for the first time, calculations of aerosol–climate interactions under Arctic conditions. Aircraft- and ground-based measurements were used to better establish the BC source regions that supply the Arctic via long-range transport mechanisms, with evidence for a dominant springtime contribution from eastern and southern Asia to the middle troposphere, and a major contribution from northern Asia to the surface. (4) Measurements of ice nucleating particles (INPs) in the Arctic indicate that a major source of these particles is mineral dust, likely derived from local sources in the summer and long-range transport in the spring. In addition, INPs are abundant in the sea surface microlayer in the Arctic, and possibly play a role in ice nucleation in the atmosphere when mineral dust concentrations are low. (5) Amongst multiple aerosol components, BC was observed to have the smallest effective deposition velocities to high Arctic snow (0.03 cm s−1).